Supplementary data for the article "Doping-control of excitons and magnetism in few-layer CrSBr"

Zitation: Tabataba-Vakili, Farsane und Baimuratov, Anvar und Högele, Alexander: Supplementary data for the article "Doping-control of excitons and magnetism in few-layer CrSBr". 8. März 2024. Open Data LMU. 10.5282/ubm/data.450

Be­schrei­bung

Magnetism in two-dimensional materials reveals phenomena distinct from bulk magnetic crystals, with sensitivity to charge doping and electric fields in monolayer and bilayer van der Waals magnet CrI3. Within the class of layered magnets, semiconducting CrSBr stands out by featuring stability under ambient conditions, correlating excitons with magnetic order and thus providing strong magnon-exciton coupling, and exhibiting peculiar magneto-optics of exciton-polaritons. Here, we demonstrate that both exciton and magnetic transitions in bilayer and trilayer CrSBr are sensitive to voltage-controlled field-effect charging, exhibiting bound exciton-charge complexes and doping-induced metamagnetic transitions. Moreover, we demonstrate how these unique properties enable optical probes of local magnetic order, visualizing magnetic domains of competing phases across metamagnetic transitions induced by magnetic field or electrostatic doping. Our work identifies few-layer CrSBr as a rich platform for exploring collaborative effects of charge, optical excitations, and magnetism.

• Dokumententyp: Daten
• Name der Kontakt­person: Tabataba-Vakili, Farsane
• E-Mail der Kontaktperson: f.tabataba at physik.uni-muenchen.de
• Fächer: Physik
• Dewey Dezimal­klassi­fikation: 500 Naturwissenschaften und Mathematik ; 500 Naturwissenschaften und Mathematik > 530 Physik
• Eingestellt von: Dr. Farsane Tabataba-Vakili